最初のカウントをサブクエリに入れる必要があります:
SELECT COUNT(CASE WHEN C = 1 THEN 1 END) AS nooffamiliesHavingcount1,
COUNT(CASE WHEN C = 2 THEN 1 END) AS nooffamiliesHavingcount2
FROM ( SELECT COUNT(*) AS C
FROM TableName
GROUP BY House_No
) t
WHERE c IN (1, 2);
編集
カウントで範囲を設定する必要がある場合は、次を使用できます:
SELECT COUNT(CASE WHEN C <= 1 THEN 1 END) AS nooffamiliesHavingcount1,
COUNT(CASE WHEN C BETWEEN 2 AND 4 THEN 1 END) AS nooffamiliesHavingcount2,
COUNT(CASE WHEN C > 4 THEN 1 END) AS nooffamiliesHavingcount3
FROM ( SELECT COUNT(*) AS C
FROM TableName
GROUP BY House_No
) t